TANDEM IN SITU SYNTHESIS AND REARRANGEMENT OF CERTAIN HYDRAZONATE ESTERS

Thoraya Abd El Reheem Farghaly Mohamed;

Abstract


The first part of the original work of the thesis outlines a facile one­ pot regioselective synthesis of [I ,2,4]triazolo[4,3-a]-5(1 H)-pyrimidinones via tandem Japp-Kiingemann, Smiles rearrangement and cyclization
reactions by azo coupling of various diazonium salts with the respective
I substitution products obtained from reaction of6-phenyl-2-thiouracil with ,
some active chloromethylene compounds.

The second part deals with synthesis offunctionalized derivatives of novel pentaheterocyclic ring system namely pyrido[2,3-f: 6,5-f •]di- [1 ,2,4]triazolo[4,3-a]pyrimidin-5(1H)-one. The synthetic strategy is based

1 on

reaction odf hy_drazonoyl haflid es witdh dpyridodipy •imbidi nes. Th e .

mec 1hanisms an regiochemistry of the studies reactions in both resesrch
projects were discussed.


Other data

Title TANDEM IN SITU SYNTHESIS AND REARRANGEMENT OF CERTAIN HYDRAZONATE ESTERS
Other Titles الاصطناع والتعديل الجزيئي المتتابعان داخليا لبعض أسترات هيدرازونوات
Authors Thoraya Abd El Reheem Farghaly Mohamed
Issue Date 2001

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